I've been using BeInSync (http://www.beinsync.com) lately to keep my files in sync between the different computers I'm using. It was also extremely helpful when I got a new laptop and had to migrate the data from the old laptop to the new one.
I recently came across MoveIt, which is more of a solution for the IT pros who wish to migrate PCs and transfer files between them. Check out SpearIt (http://www.spearit.com) for more information.
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